You have to create a simulator using the simulator os version. You have only downloaded the iOS version software.
To add a device follow: Window > Devices & Simulators. (or cmd + shift + 2)
Then at the bottom of the list press the + icon. This should allow you to add a device running the selected iOS version.
iOS 9.3 (9.3 - 13E233) - com.apple.CoreSimulator.SimRuntime.iOS-9-3(不可用,macOS 10.14.99 之后的主机不支持 iOS 9.3 模拟器运行时。)(不可用,iOS 9.3 模拟器运行时是macOS 10.14.99 之后的主机不支持。)
Keep the Deployment Targets at 9.x, then navigate to:
Xcode > Preferences > Components
There you will see a list of additional simulators to install. These can sometimes take an really long time to download, and I've found this article to be very helpful in speeding up the process.
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